I taped the mold in place over the gap, trying to align all the surface detail. Then I mixed some "hard plaster" and poured that into the opening. I probably should have gone with some kind of resin, but the plaster was what I had lying around.
My first attempt was too thin and brittle and the mold was not tightly secured. If you pour 2-3mm of plaster, you end up with a cast of about 1-2mm since all the particles sink to the bottom and the water evaporates.
On the second attempt, I doubled the amount, which turned out as I wanted it.
First attempt Second attempt
Now I just need to fill the gaps and see how well it responds to paint.
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